Passivation Using Molecular Halides Increases Quantum Dot Solar Cell Performance.

نویسندگان

  • Xinzheng Lan
  • Oleksandr Voznyy
  • Amirreza Kiani
  • F Pelayo García de Arquer
  • Abdullah Saud Abbas
  • Gi-Hwan Kim
  • Mengxia Liu
  • Zhenyu Yang
  • Grant Walters
  • Jixian Xu
  • Mingjian Yuan
  • Zhijun Ning
  • Fengjia Fan
  • Pongsakorn Kanjanaboos
  • Illan Kramer
  • David Zhitomirsky
  • Philip Lee
  • Alexander Perelgut
  • Sjoerd Hoogland
  • Edward H Sargent
چکیده

A solution-based passivation scheme is developed featuring the use of molecular iodine and PbS colloidal quantum dots (CQDs). The improved passivation translates into a longer carrier diffusion length in the solid film. This allows thicker solar-cell devices to be built while preserving efficient charge collection, leading to a certified power conversion efficiency of 9.9%, which is a new record in CQD solar cells.

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Restricted charge recombination process in PbS quantum dot sensitized solar cells by different coating cycles of ZnS films

The relatively low power conversion efficiency (PCE) of quantum dot sensitized solar cells (QDSSCs) is attributed to charge recombination at the interfaces. Charge recombination process could be suppressed by coating the QD layer with a wide band gap semiconductor such as ZnS, which acts as a blocking layer between the QDs and hole transport material (HTM). In present study, to improve PCE of P...

متن کامل

Effect of PbS Film Thickness on the Performance of Colloidal Quantum Dot Solar Cells

Colloidal quantum dots offer broad tuning of semiconductor band structure via the quantum size effect. In this paper, we present a detailed investigation on the influence of the thickness of colloidal lead sulfide (PbS) nanocrystals (active layer) to the photovoltaic performance of colloidal quantum dot solar cells. The PbS nanocrystals (QDs) were synthesized in a non-coordinating solvent, 1-oc...

متن کامل

Strategies for Performance Improvement of Quantum Dot Sensitized Solar Cells

Quantum dot sensitized solar cells (QDSCs) constitute one of the most promising low-cost solutions that currently are explored for the world’s needs of clean and renewable energy. Efficient, low-toxic and stable QDSCs for large-scale applications have therefore formed the subject for much of the solar cell research during recent years. This circumstance also forms the basic motivation f...

متن کامل

Introducing nanostructure patterns for performance enhancement in PbS colloidal quantum dot solar cells

With attention to the thin film structure of colloidal quantum dot solar cells, in this paper in order to improvement of active layer absorption of them, we have proposed the use of nanostructure pattern for enhancement of their performance. For this purpose we have presented suitable nano hemisphare patterns in colloidal quantum dot solar cells for light trapping in absorption layer. Then with...

متن کامل

SILAR Sensitization as an Effective Method for Making Efficient Quantum Dot Sensitized Solar Cells

CdSe quantum dots were in situ deposited on various structures of TiO2 photoanode by successive ionic layer adsorption and reaction (SILAR). Various sensitized TiO2 structures were integrated as a photoanode in order to make quantum dot sensitized solar cells. High power conversion efficiency was obtained; 2.89 % (Voc=524 mV, Jsc=9.78 mA/cm2, FF=0.56) for the cells that sensitized by SILAR meth...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

برای دانلود متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

عنوان ژورنال:
  • Advanced materials

دوره 28 2  شماره 

صفحات  -

تاریخ انتشار 2016